The invention provides non-aqueous decarburization solution for capturing carbon dioxide in a mixed gas, and belongs to the technical field of capturing of carbon dioxide gas. The invention relates to a non-aqueous decarburization solution, wherein a main absorption component is N-ethyldiethanolamine, and a solvent is N,N-diethylethanolamine. Because the non-aqueous decarburization solution has a high boiling point and low viscosity, uses tertiary amine capable of participating in CO2 absorption as the solvent, and uses secondary amine with a fast absorption speed and a high absorption amount, and easy to regenerate as the main absorption solvent, the absorption capacity, purification degree and desorption speed for carbon dioxide are increased, the temperature range of the reaction is expanded, the volume of a regeneration tower is reduced, the energy consumption of the regeneration is greatly reduced, and the equipment investment and operation cost are reduced. The non-aqueous decarburization solution provided by the invention is mainly used for capturing carbon dioxide in the tail gases of multiple chemical reactions, the tail gases of steel plants and cement plants, ore decomposition gas, combustion flue gas, natural gas, city gas and marsh gas, and has wide application prospect.