This invention belongs to the technical fields of optoelectronic devices, spin
optoelectronics, and organic-inorganic
hybrid semiconductor materials. Specifically, it relates to a circularly polarized electroluminescent device based on a one-dimensional / three-dimensional
perovskite heterostructure and its implementation method. The circularly polarized electroluminescent device includes a substrate, a bottom
electrode layer, an
electron transport layer, a light-emitting layer, a
hole transport layer, and a top
electrode stacked sequentially. The light-emitting layer is a one-dimensional / three-dimensional
perovskite heterostructure formed in situ by chiral one-dimensional
perovskite and three-dimensional perovskite. This invention constructs a one-dimensional / three-dimensional perovskite heterostructure within the light-emitting layer, utilizing the chiral properties of the one-dimensional perovskite to induce lattice
distortion in adjacent three-dimensional perovskite at the heterostructure interface. This results in intrinsic structural
chirality and excited-state
chirality in the three-dimensional perovskite light-emitting region, achieving stable circularly polarized
electroluminescence without the need for an external
magnetic field or
spin injection, thus enabling the device to simultaneously achieve high luminous efficiency and good stability.