The invention belongs to the field of
graphene preparation, and discloses a
graphene cement additive and a preparation method thereof, and a
graphene-
cement composite material and a preparation method thereof. The preparation method comprises the following steps: preparing a stripping agent solution from pure water, a cholate anionic surfactant and a
nonionic surfactant, then adding a
graphite raw material, and fully stirring and mixing to obtain a
graphite pre-stripping dispersion liquid; performing auxiliary stripping dispersion on the
graphite pre-stripping dispersion liquid through water bath ultrasonic to obtain a graphene mixed dispersion
system: centrifuging the graphene mixed dispersion
system, taking an upper-layer solution for
dialysis, and removing unstripped particles or thick graphite flakes to obtain the graphene
cement additive. According to the graphene cement additive, pure water is used as a stripping agent, the graphene cement additive is directly obtained by adding a small amount of surfactant and
liquid phase stripping, the graphene cement additive is non-toxic and harmless, the
dispersity of obtained graphene is good, and after the graphene cement additive is blended into cement, the
compressive strength of the cement is improved by 20% or above.